All-optical measurement of magnetic fields for quantum gas experiments.

We present an all-optical method to measure and compensate for residual magnetic fields present in a cloud of ultracold atoms trapped in an optical dipole trap. Our approach leverages the increased loss from the trapped atomic sample through electromagnetically induced absorption. Modulating the excitation laser provides coherent sidebands, resulting in a Λ-type pump-probe scheme. Scanning an additional magnetic offset field leads to pairs of sub-natural linewidth resonances, whose positions encode the magnetic field in all three spatial directions. Our measurement scheme is readily implemented in typical quantum gas experiments and has no particular hardware requirements.

Exploring the vibrational series of pure trilobite Rydberg molecules.

In trilobite Rydberg molecules, an atom in the ground state is bound by electron-atom scattering to a Rydberg electron that is in a superposition of high angular momentum states. This results in a homonuclear molecule with a permanent electric dipole moment in the kilo-debye range. Trilobite molecules have previously been observed only with admixtures of low-l states. Here we report on the observation of two vibrational series of pure trilobite Rubidium-Rydberg molecules that are nearly equidistant. They are produced by three-photon photoassociation and lie energetically more than 15 GHz below the atomic 22F state of rubidium. We show that these states can be used to measure the electron-atom scattering length at low energies in order to benchmark current theoretical calculations. In addition to measuring their kilo-Debye dipole moments, we also show that the molecular lifetime is increased compared to the 22F state due to the high-l character. The observation of an equidistant series of vibrational states opens the way to observe coherent molecular wave packet dynamics.

Kapitza Trap for Ultracold Atoms.

We report on the experimental realization of a Kapitza trap for ultracold atoms. Using time-periodic attractive and repulsive Gaussian potentials, we create an effective trap for ultracold neutral atoms in a regime where the time average of the potential is equal to zero. We analyze the role of experimental imperfections, the stability of the trapped atomic cloud, and the magnitude of the effective potential. We find good agreement with the high-frequency expansion of the underlying system dynamics. Our experimental approach opens up new possibilities to study Floquet systems of neutral atoms.

Experimental realization of a 3D random hopping model.

Scientific advance is often driven by identifying conceptually simple models underlying complex phenomena. This process commonly ignores imperfections which, however, might give rise to non-trivial collective behavior. For example, already a small amount of disorder can dramatically change the transport properties of a system compared to the underlying simple model. While systems with disordered potentials were already studied in detail, experimental investigations on systems with disordered hopping are still in its infancy. To this end, we experimentally study a dipole-dipole-interacting three-dimensional Rydberg system and map it onto a simple XY model with random couplings by spectroscopic evidence. We discuss the localization-delocalization crossover emerging in the model and present experimental signatures of it. Our results demonstrate that Rydberg systems are a useful platform to study random hopping models with the ability to access the microscopic degrees of freedom. This will allow to study transport processes and localization phenomena in random hopping models with a high level of control.

Diffusive-like redistribution in state-changing collisions between Rydberg atoms and ground state atoms.

Exploring the dynamics of inelastic and reactive collisions on the quantum level is a fundamental goal in quantum chemistry. Such collisions are of particular importance in connection with Rydberg atoms in dense environments since they may considerably influence both the lifetime and the quantum state of the scattered Rydberg atoms. Here, we report on the study of state-changing collisions between Rydberg atoms and ground state atoms. We employ high-resolution momentum spectroscopy to identify the final states. In contrast to previous studies, we find that the outcome of such collisions is not limited to a single hydrogenic manifold. We observe a redistribution of population over a wide range of final states. We also find that even the decay to states with the same angular momentum quantum number as the initial state, but different principal quantum number is possible. We model the underlying physical process in the framework of a short-lived Rydberg quasi-molecular complex, where a charge exchange process gives rise to an oscillating electric field that causes transitions within the Rydberg manifold. The distribution of final states shows a diffusive-like behavior.

Coherent perfect absorber and laser for nonlinear waves in optical waveguide arrays.

A localized non-Hermitian potential can operate as a coherent perfect absorber or as a laser for nonlinear waves. The effect is illustrated for an array of optical waveguides, with the central waveguide being either active or absorbing. The arrays situated to the left and to the right of the center can have different characteristics. The result is generalized to setups with the central waveguide carrying additional nonlinear dissipation or gain and to the two-dimensional arrays with embedded one-dimensional absorbing or lasing subarrays.

Coherent perfect absorption of nonlinear matter waves.

Coherent perfect absorption is the complete extinction of incoming radiation by a complex potential in a physical system supporting wave propagation. The concept was proven for linear waves in a variety of systems including light interacting with absorbing scatterers, plasmonic metasurfaces, and graphene films, as well as sound waves. We extend the paradigm to coherent perfect absorption of nonlinear waves and experimentally demonstrate it for matter waves in an atomic Bose-Einstein condensate. Coherent absorption of nonlinear matter waves is achieved easier than its linear analogs because the strength of two-body interactions offers additional freedom for control. Implementation of the coherent perfect absorber of Bose-Einstein condensates paves the way toward broad exploitation of the phenomenon in nonlinear optics, exciton-polariton condensates, acoustics, and other areas of nonlinear physics. It also opens perspectives for designing atom lasers.

Measuring finite-range phase coherence in an optical lattice using Talbot interferometry.

One of the important goals of present research is to control and manipulate coherence in a broad variety of systems, such as semiconductor spintronics, biological photosynthetic systems, superconducting qubits and complex atomic networks. Over the past decades, interferometry of atoms and molecules has proven to be a powerful tool to explore coherence. Here we demonstrate a near-field interferometer based on the Talbot effect, which allows us to measure finite-range phase coherence of ultracold atoms in an optical lattice. We apply this interferometer to study the build-up of phase coherence after a quantum quench of a Bose-Einstein condensate residing in a one-dimensional optical lattice. Our technique of measuring finite-range phase coherence is generic, easy to adopt and can be applied in practically all lattice experiments without further modifications.

Rydberg Molecule-Induced Remote Spin Flips.

We have performed high resolution photoassociation spectroscopy of rubidium ultralong-range Rydberg molecules in the vicinity of the 25P state. Because of the hyperfine interaction in the ground state perturber atom, the emerging mixed singlet-triplet potentials contain contributions from both hyperfine states. We show that this can be used to induce remote spin flips in the perturber atom upon excitation of a Rydberg molecule. Furthermore, when the spin-orbit splitting of the Rydberg state is comparable to the hyperfine splitting in the ground state, the orbital angular momentum of the Rydberg electron is entangled with the nuclear spin of the perturber atom. Our results open new possibilities for the implementation of spin-dependent interactions for ultracold atoms in bulk systems and in optical lattices.

Observation of pendular butterfly Rydberg molecules.

Engineering molecules with a tunable bond length and defined quantum states lies at the heart of quantum chemistry. The unconventional binding mechanism of Rydberg molecules makes them a promising candidate to implement such tunable molecules. A very peculiar type of Rydberg molecules are the so-called butterfly molecules, which are bound by a shape resonance in the electron-perturber scattering. Here we report the observation of these exotic molecules and employ their exceptional properties to engineer their bond length, vibrational state, angular momentum and orientation in a small electric field. Combining the variable bond length with their giant dipole moment of several hundred Debye, we observe counter-intuitive molecules which locate the average electron position beyond the internuclear distance.

Bistability in a Driven-Dissipative Superfluid.

We experimentally study a driven-dissipative Josephson junction array, realized with a weakly interacting Bose-Einstein condensate residing in a one-dimensional optical lattice. Engineered losses on one site act as a local dissipative process, while tunneling from the neighboring sites constitutes the driving force. We characterize the emerging steady states of this atomtronic device. With increasing dissipation strength γ the system crosses from a superfluid state, characterized by a coherent Josephson current into the lossy site, to a resistive state, characterized by an incoherent hopping transport. For intermediate values of γ, the system exhibits bistability, where a superfluid and an incoherent branch coexist. We also study the relaxation dynamics towards the steady state, where we find a critical slowing down, indicating the presence of a nonequilibrium phase transition.

Single atom detection in ultracold quantum gases: a review of current progress.

The recent advances in single atom detection and manipulation in experiments with ultracold quantum gases are reviewed. The discussion starts with the basic principles of trapping, cooling and detecting single ions and atoms. The realization of single atom detection in ultracold quantum gases is presented in detail and the employed methods, which are based on light scattering, electron scattering, field ionization and direct neutral particle detection are discussed. The microscopic coherent manipulation of single atoms in a quantum gas is also covered. Various examples are given in order to highlight the power of these approaches to study many-body quantum systems.

Negative Differential Conductivity in an Interacting Quantum Gas.

We report on the observation of negative differential conductivity (NDC) in a quantum transport device for neutral atoms employing a multimode tunneling junction. The system is realized with a Bose-Einstein condensate loaded in a one-dimensional optical lattice with high site occupancy. We induce an initial difference in chemical potential at one site by local atom removal. The ensuing transport dynamics are governed by the interplay between the tunneling coupling, the interaction energy, and intrinsic collisions, which turn the coherent coupling into a hopping process. The resulting current-voltage characteristics exhibit NDC, for which we identify atom number-dependent tunneling as a new microscopic mechanism. Our study opens new ways for the future implementation and control of complex neutral atom quantum circuits.

Giant Cross Section for Molecular Ion Formation in Ultracold Rydberg Gases.

We have studied the associative ionization of a Rydberg atom and a ground-state atom in an ultracold Rydberg gas. The measured scattering cross section is 3 orders of magnitude larger than the geometrical size of the produced molecule. This giant enhancement of the reaction kinetics is due to an efficient directed mass transport which is accelerated by the Rydberg electron. We also find that the total inelastic scattering cross section is given by the geometrical size of the Rydberg electron's wave function.

Dimensional phase transition from an array of 1D Luttinger liquids to a 3D Bose-Einstein condensate.

We study the thermodynamic properties of a 2D array of coupled one-dimensional Bose gases. The system is realized with ultracold bosonic atoms loaded in the potential tubes of a two-dimensional optical lattice. For negligible coupling strength, each tube is an independent weakly interacting 1D Bose gas featuring Tomonaga Luttinger liquid behavior. By decreasing the lattice depth, we increase the coupling strength between the 1D gases and allow for the phase transition into a 3D condensate. We extract the phase diagram for such a system and compare our results with theoretical predictions. Because of the high effective mass across the periodic potential and the increased 1D interaction strength, the phase transition is shifted to large positive values of the chemical potential. Our results are prototypical to a variety of low-dimensional systems, where the coupling between the subsystems is realized in a higher spatial dimension such as coupled spin chains in magnetic insulators.

Observation of local temporal correlations in trapped quantum gases.

We measure the temporal pair correlation function g(2)(τ) of a trapped gas of bosons above and below the critical temperature for Bose-Einstein condensation. The measurement is performed in situ by using a local, time-resolved single-atom sensitive probing technique. Third- and fourth-order correlation functions are also extracted. We develop a theoretical model and compare it with our experimental data, finding good quantitative agreement. We discuss, finally, the role of interactions. Our results promote temporal correlations as new observables to study the dynamical evolution of ultracold quantum gases.

Experimental demonstration of single-site addressability in a two-dimensional optical lattice.

We demonstrate single-site addressability in a two-dimensional optical lattice with 600 nm lattice spacing. After loading a Bose-Einstein condensate in the lattice potential, we use a focused electron beam to remove atoms from selected sites. The patterned structure is subsequently imaged by means of scanning electron microscopy. This technique allows one to create arbitrary patterns of mesoscopic atomic ensembles. We find that the patterns are remarkably stable against tunneling diffusion. Such microengineered quantum gases are a versatile resource for applications in quantum simulation, quantum optics, and quantum information processing with neutral atoms.

Dissipation-induced coherent structures in Bose-Einstein condensates.

We discuss how to engineer the phase and amplitude of a complex order parameter using localized dissipative perturbations. Our results are applied to generate and control various types of atomic nonlinear matter waves (solitons) by means of localized dissipative defects.